Mr. Ice and his henchman Freezer Freezer freeze the city in order to take it over.

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Dr. Spectro creates three giant ghoulish ghosts in order to take over Penciltrainia.

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The Batter kidnaps a baseball star and holds him for ransom.

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Mr. Instant uses his insta-gun that can make anything in an instant.

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Mr. Menace uses his putty monster to steal a $1,000,000 coin collection and even kidnaps Buzz. It is up to Frankenstein Jr. to rescue Buzz and defeat Mr. Menace.

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The Clutcher uses an invention that brings his gloves to life.

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Dr. Futuro comes from the 40th century to the twentieth century to steal a million dollar gold brick.

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The Mad Inventor has invented the Monstermobile and uses its many gadgets to commit crimes.

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Billy the Kidder is a cowboy who rides a robotic horse and plans to rob the U.S. Mint.

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The Ringmaster puts on a circus and robs from those who attend.

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To perform a crime wave in London, Baron Von Ghoul creates robotic versions of the horror movie monsters the Electroflying Firefly, the Menacing Mummy, and the Wicked Werewolf.

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The Angler steals secret space research.

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The Tapper transmits himself over phone lines.

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Professor Stretch returns and creates a rubber monster to help him.

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The Twister is stealing precious jewels.

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Sertano the Satellite King, an alien from Galaxy X, uses a gravity ray in order to get Earth to surrender. Buzz and Frankenstein Jr. must defeat Sertano's robots in order to defeat him.

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A witch named Cronella Critch robs a charity for orphans party.

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The Paper Doll Man returns and causes trouble.

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Birdman and his robotic birds Vulturo, Rodantus, and King Condor abduct two astronauts and hold them for a ransom of $1,000,000.

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The Diamond Dazzler steals a precious diamond in order to awaken the genie within.

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The Inflator creates giant balloon monsters to help him commit crimes.

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Zorbo the Great creates a genie and plans to use its three wishes in order to defeat Frankenstein Jr. and conquer the world.

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The Archer steals a priceless violin and a million dollars.

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The Sculptor turns people into statues.

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Buzz and Frankenstein Jr. guard the Navy's new Hydrotomic Submarine to prevent Dr. Hook and his aquatic monsters from stealing it.

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Spraysol steals top secret documents.

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The Junk Man creates the Colossal Junk Monster in a plot to eliminate Frankenstein Jr.

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The Surfer takes pictures of a top secret submarine.

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The Spinner returns and steals a priceless pooch.

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The Mad Inventor has invented the Double Identity Duplicator Projector to create living images he can control.

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The Dragster has stolen a valuable item.

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Professor Stretch causes havoc with his elastic abilities.

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Plant Man thaws the last three prehistoric plants (the Carnivorous Chewer, the Creeping Crusher and the Fire-Breathing Snapdragon) from a glacier and then sprays them with his Obedience Ray in a plot to eliminate Buzz and Frankenstein Jr.

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Aquator has stolen a secret formula from a scientist who is friends with Big D and shrinks himself to microscopic size in order to get all the microscopic creatures to become large.

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The Dauber uses a special brush where anything he paints becomes real.

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The alien Zargon unleashes his warrior Destructo to conquer Earth.

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Televisatron transports the Impossibles to different television shows.

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Mother Gruesome invents a machine that brings villainous storybook characters out of their stories to help her with her crimes.

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A giant alien brain arrives on Earth and captures Buzz and Frankenstein Jr.

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To get the Impossibles out of the way, Fero uses his fiddle to transport them to different planets.

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The Speck uses a formula to shrink himself in order to photograph top secret plans.

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A giant alien brain arrives on Earth and captures Buzz and Frankenstein Jr.

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Smogula freezes the Impossibles and seals them within a cave, so they will not interfere with his plans to conquer Empire City.

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Timeatron uses his time cabinet to bring villains from the past to pillage for him.

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Upon an encounter with Buzz at the wax museum, Mr. Menace uses his monsters Godzonka, Gorillis and Cyclaws in an attack upon San Francisco.

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The Burrower uses his burrowing machine to steal half a million dollars from the bank and dig ten miles down to his lair.

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Beamatron steals a priceless painting from a ship.

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Professor Conroy and Buzz unveil the blueprints for the Spy Detector XK-00-7 at a Maximum Security Building. Unfortunately, the blueprints are targeted by the Spyder Man.

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The Paper Doll Man steals a top secret plan and is out to steal the second part.

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The Spinner steals a $1,000,000 tiara.

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Dr. Shock uses his Master Mix Monster Machine to turn his assistant Igor into an electricity-absorbing monster.

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The Bubbler kidnaps the Shah of Shish-Ka-Bob and it's up to the Impossibles to rescue him.

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